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Journal Articles

Irradiation behavior of rock-like oxide fuels

Yamashita, Toshiyuki; Kuramoto, Kenichi; Shirasu, Noriko; Nakano, Yoshihiro; Akie, Hiroshi; Nagashima, Hisao; Kimura, Yasuhiko; Omichi, Toshihiko*

Journal of Nuclear Materials, 320(1-2), p.126 - 132, 2003/07

 Times Cited Count:10 Percentile:56.43(Materials Science, Multidisciplinary)

Two irradiation tests on the rock-like oxide (ROX) fuels, small disk-shape fuel targets and pellet-type fuels, were performed in order to clarify in-pile irradiation stabilities. Swelling, fractional fission gas release (FGR) and phase change were examined by puncture test, profilometry and ceramography. YSZ single-phase fuel showed an excellent irradiation behavior, ie. low fission gas release (less than 3%), negligible swelling and no appreciable restructuring. The particle dispersed fuels showed lower swelling and higher fission gas release than those of mechanically blended fuels. Spinel decomposition and subsequence restructuring in the spinel matrix fuels was observed for the first time in the present investigation. It would be possible to reduce the FGR of the spinel matrix fuels, if the maximum fuels temperature is limited below 1700 K where neither spinel decomposition nor restructuring was observed. Damaged area of spinel matrix due to fission fragment irradiation seemed to be confined to thin layers around the surface of YSZ particles.

Journal Articles

Morphology change of rock-like oxide fuels in reactivity-initiated-accident simulation tests

Nakamura, Takehiko; Sasajima, Hideo; Yamashita, Toshiyuki; Uetsuka, Hiroshi

Journal of Nuclear Materials, 319, p.95 - 101, 2003/06

 Times Cited Count:2 Percentile:19(Materials Science, Multidisciplinary)

Pulse irradiation tests under simulated RIA conditions were performed with three types of ROX fuels. Single phase YSZ, homogeneous mixture of YSZ/spinel and YSZ particle dispersed in spinel type ROX fuels were pulse irradiated in the Nuclear Safety Research Reactor (NSRR). Mode and threshold of the fuel failure including its consequences were investigated under the RIA conditions. The fuel failure occurred in a burst type mode in all the three types of ROX fuel tests with considerable fuel melting. Even though the mode was quite different from those of UO$$_{2}$$ fuel, failure threshold enthalpies of the ROX fuels were close to that of UO$$_{2}$$ fuel at about 10 GJ m$$^{-3}$$. The consequence of the failure of the ROX fuels was different from the one of UO$$_{2}$$ fuel, because molten fuel dispersal occurred at lower enthalpies in the ROX fuel tests. Change of the fuel structure and material interaction in the transient heating conditions were examined through optical and secondary electron microscopy, and electron probe micro analysis.

Journal Articles

Behavior of YSZ based rock-like oxide fuels under simulated RIA conditions

Nakamura, Takehiko; Kusagaya, Kazuyuki*; Sasajima, Hideo; Yamashita, Toshiyuki; Uetsuka, Hiroshi

Journal of Nuclear Science and Technology, 40(1), p.30 - 38, 2003/01

 Times Cited Count:4 Percentile:31.64(Nuclear Science & Technology)

Pulse irradiation tests of three types of ROX fuel, i.e. YSZ single phase, finely mixed two phase composite of YSZ and spinel, and the other composite of larger YSZ particles dispersed in spinel matrix, were conducted in the NSRR to investigate their behavior under RIA conditions. Owing to their lower melting temperatures than that of UO$$_{2}$$ fuel, melting of ROX fuel occurred while the cladding was still solid and intact in the accident conditions. Therefore, consequence of the ROX fuel failure was quite different from that of UO$$_{2}$$ fuel. When the ROX fuels failed, a considerable amount of the molten fuel was released out to the surrounding coolant water. In spite of the release, no significant mechanical energy generation due to fuel/coolant thermal interaction was observed in the tested enthalpy range below 12 GJ/m$$^{3}$$. In terms of the failure threshold, on the other hand, the ROX fuels failed at fuel volumetric enthalpies above 10 GJ/m$$^{3}$$, which was comparable to that of UO$$_{2}$$ fuel. The results highlighted controlling parameters on the fuel behavior under the RIA conditions.

Journal Articles

Rock-like oxide fuels and their burning in LWRs

Yamashita, Toshiyuki; Kuramoto, Kenichi; Akie, Hiroshi; Nakano, Yoshihiro; Shirasu, Noriko; Nakamura, Takehiko; Kusagaya, Kazuyuki*; Omichi, Toshihiko*

Journal of Nuclear Science and Technology, 39(8), p.865 - 871, 2002/08

 Times Cited Count:25 Percentile:81.52(Nuclear Science & Technology)

Research on the plutonium rock-like oxide (ROX) fuels and their once-through burning in light water reactors has been performed to establish an option for utilizing and disposing effectively the excess plutonium. The ROX fuel is a sort of the inert matrix fuels and consists of mineral-like compounds such as yttria stabilized zirconia, spinel and corundum. A particle-dispersed fuel was devised to reduce damage by heavy fission fragments. Some preliminary results on swelling, fractional gas release and microstructure change for five ROX fuels were obtained from the irradiation test and successive post-irradiation examinations. Inherent disadvantages of the Pu-ROX fuel cores could be improved by adding 238U or 232Th as resonant materials, and all improved cores showed a nearly the same characteristics as the conventional UO2 core during transient conditions. The threshold enthalpy of the ROX fuel rod failure was found to be comparable to the fresh UO2 rod by pulse-irradiation tests simulating reactivity initiated accident conditions.

Journal Articles

A Study of actinide decay chains on the environmental effect of a geologic disposal of rock-like oxide fuels and uranium-plutonium oxide fuels

Kimura, Hideo; Takano, Hideki; Muromura, Tadasumi

Journal of Nuclear Materials, 274(1-2), p.197 - 205, 1999/00

 Times Cited Count:7 Percentile:49.7(Materials Science, Multidisciplinary)

no abstracts in English

JAEA Reports

Environmental safety of the geologic disposal of ROX and MOX spent-fuels

Kimura, Hideo; Matsuzuru, Hideo; Takano, Hideki; Muromura, Tadasumi

JAERI-Research 97-049, 25 Pages, 1997/07

JAERI-Research-97-049.pdf:1.42MB

no abstracts in English

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